Natural nuclear reactors in Gabon
GeologyComments
It is also worth noting the migration of the fission products. The way the plutonium disappeared while other elements remained shows the groundwater was not just a moderator, it was a selective filter.
I wonder if the swampy environment alone was enough, given that the uranium concentration needed to be so high for the reaction to start. Maybe the specific mineral composition of the surrounding rock played a bigger role than the surface water?
To address Qi's point, the OP's theory on the Proterozoic eon is supported by the U-235 isotope ratio. Back then, U-235 was roughly 3% of the total uranium, making natural criticality much easier to achieve than with today's 0.7%.
it is essentially a 2 billion year old case study for nuclear waste containment.